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If it still won't sync, go into itunes, find the album you are wanting artwork for and copy the exact name of it into the details of the uploaded album. If the artist/album doesn't match perfect the artwork won't always sync properly
You can do it manually by selecting all the songs in the album, then right click and 'get info'
Go to the info tab and it'll have a box where you can just drag a pic from your pc into itunes. if you dont have the artwork just google it. i get a lot off amazon.